Research Article
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Review of the vapour pressures of ice and supercooled water for atmospheric applications

D. M. Murphy

Corresponding Author

E-mail address:daniel.m.murphy@noaa.gov

Aeronomy Laboratory, National Oceanic and Atmospheric Administration, Boulder, USA

Aeronomy Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA.
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T. Koop

University of Bielefeld, Faculty of Chemistry, Germany

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First published: 29 December 2006
Cited by: 416

Abstract

The vapour pressures of ice and supercooled water are reviewed with an emphasis on atmospheric applications. Parametrizations are given for the vapour pressure, molar heat capacity, and latent heat of vaporization of both ice and liquid water. For ice, the experimental vapour pressure data are in agreement with a derivation from the Clapeyron equation. Below 200 K cubic ice may affect the vapour pressure of ice both in the atmosphere and in the laboratory. All of the commonly used parametrizations for the vapour pressure of supercooled water are extrapolations that were not originally intended for use below the freezing point. In addition, the World Meteorological Organization definition of the vapour pressure of supercooled water contains an easily overlooked typographical error. Recent data on the molar heat capacity of supercooled water are used to derive its vapour pressure. Nevertheless, the uncertainty is such that measurements of the deliquescence and freezing behaviour of aerosol particles are beginning to be limited by uncertainties in the thermodynamics of supercooled water. Copyright © 2005 Royal Meteorological Society

Number of times cited: 416

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  • , Assessment of NASA GISS CMIP5 and Post-CMIP5 Simulated Clouds and TOA Radiation Budgets Using Satellite Observations. Part I: Cloud Fraction and Properties, Journal of Climate, 10.1175/JCLI-D-13-00558.1, 27, 11, (4189-4208), (2014).
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  • , Bounding the role of black carbon in the climate system: A scientific assessment, Journal of Geophysical Research: Atmospheres, 118, 11, (5380-5552), (2013).
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  • , Site selection for a radio astronomy observatory in Turkey: atmospherical, meteorological, and radio frequency analyses, Experimental Astronomy, 33, 1, (1), (2012).
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  • , Initial Ice Microparticle Sublimation Measurements from the Levitating Upper-Tropospheric Environmental Simulator (LUTES), Journal of Atmospheric and Oceanic Technology, 28, 7, (884), (2011).
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  • , Seasonal to decadal variations of water vapor in the tropical lower stratosphere observed with balloon‐borne cryogenic frost point hygrometers, Journal of Geophysical Research: Atmospheres, 115, D18, (2010).
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  • , Effects of sulfate coatings on the ice nucleation properties of a biological ice nucleus and several types of minerals, Journal of Geophysical Research: Atmospheres, 115, D20, (2010).
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  • , Numerical simulations of the three‐dimensional distribution of polar mesospheric clouds and comparisons with Cloud Imaging and Particle Size (CIPS) experiment and the Solar Occultation For Ice Experiment (SOFIE) observations, Journal of Geophysical Research: Atmospheres, 115, D10, (2010).
  • , Rocket‐borne in situ measurements of meteor smoke: Charging properties and implications for seasonal variation, Journal of Geophysical Research: Atmospheres, 115, D1, (2010).
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  • , Homogeneous water nucleation and droplet growth in methane and carbon dioxide mixtures at 235 K and 10 bar, The Journal of Chemical Physics, 132, 20, (204504), (2010).
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  • , A Classical-Theory-Based Parameterization of Heterogeneous Ice Nucleation by Mineral Dust, Soot, and Biological Particles in a Global Climate Model, Journal of the Atmospheric Sciences, 10.1175/2010JAS3425.1, 67, 8, (2483-2503), (2010).
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  • , The Transition to Strong Convection, Journal of the Atmospheric Sciences, 10.1175/2009JAS2962.1, 66, 8, (2367-2384), (2009).
  • , The University of Toronto Continuous Flow Diffusion Chamber (UT-CFDC): A Simple Design for Ice Nucleation Studies, Aerosol Science and Technology, 43, 7, (730), (2009).
  • , Heat capacities of freely evaporating charged water clusters, The Journal of Chemical Physics, 130, 22, (224308), (2009).
  • , How Well Does Water Activity Determine Homogeneous Ice Nucleation Temperature in Aqueous Sulfuric Acid and Ammonium Sulfate Droplets?, Journal of the Atmospheric Sciences, 10.1175/2008JAS2542.1, 66, 3, (741-754), (2009).
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  • 44th AIAA Aerospace Sciences Meeting and Exhibit Reno, Nevada 09 January 2006 - 12 January 2006 44th AIAA Aerospace Sciences Meeting and Exhibit American Institute of Aeronautics and Astronautics Reston, Virigina , (2006). , (2012). 978-1-62410-039-0 10.2514/MASM06 , 10.2514/MASM06 2016101702455000193 http://arc.aiaa.org/doi/book/10.2514/MASM06 Large Eddy Simulation of Early Stage Contrails: Effect of Atmospheric Properties , (2006). , (2012). 10.2514/6.2006-1414 , 10.2514/6.2006-1414 2016101702455000193 http://arc.aiaa.org/doi/10.2514/6.2006-1414
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